Ukrainian Journal of Physical Optics 

Home page
 
 

Other articles 

in this issue
The Influence of Point Defects on the Vibrational Spectrum of Li2B4O7 Crystal  
1Moiseyenko V.N., 1Dergachov M.P., 2Burak Ya.V.

1Physics Department, Dnipropetrovsk National University, 13 Naukova St., 49050 Dnipropetrovsk, Ukraine
2Physical Optics Institute, 23 Dragomanov St., 79005 Lviv, Ukraine

download full version

The Raman and infrared reflection spectra of Li2B4O7 crystals doped with potassium, silver and copper ions are measured at 300 K. The damping increase of the Raman lines and the changes in the oscillator strengths for a number of reflection bands are observed in the doped crystals. The results obtained due to theoretical fitting of the spectra are discussed in the framework of heavy isotopic impurity model. The analysis of the experimental and theoretical data has allowed to assume that the potassium and silver ions represent substitution impurities, while the copper ions are probably the interstitial ones.

Keywords: Raman scattering, infrared reflection, impurity effect

PACS: 78.30.Am
Ukr. J. Phys. Opt. 7 35-40 doi: 10.3116/16091833/7/1/35/2006
Received: 20.12.2005

REFERENCES

1. Shiosaki T, Adachi M and Kawabata A 1986. IEEE Proc. 455.
2. Petrov V, Rotermund AF, Noack F, Komatsu R, 1998. J. Appl. Phys. 84: 5887.
        doi:10.1063/1.368904 http://dx.doi.org/10.1063/1.368904
3. Winogradov EL, Widay YuT, Zaganriy LB, Kudin AM, Levin AB, Nazarenko BP, Tarasov BP and Tschernikov WW, 1994. Functional Materials 1: 152.
4. Adamiv VT, Burak YaV, Kityk IV, Kasperczyk J, Smok R and Czerwinski M, 1997. Opt. Mater. 8: 207.
        doi:10.1016/S0925-3467(97)00017-7 http://dx.doi.org/10.1016/S0925-3467(97)00017-7
5. Dergachov MP, Moiseyenko VN and Burak YaV, 2001. Opt. Spektr. 90: 604.
6. Burak YaV, Tratsh IB, Adamiv VT and Teslyuk IM, 2002. Ukr. Fiz. Zhurn. 47: 923.
7. Moiseyenko VN, Vdovin AV and Burak YaV, 1996. Opt. Spektr. 81: 620.
8. Zhyzin GN, Mavrin BN and Shabanov VF, 1984. Optical vibrational spectra of crystals. Nauka. Moscow.
9. Vdovin AV, Moiseyenko VN, Gorelik VS and Burak YaV, 2001. Fizyka Tverd. Tela, 43: 1584.
10. Pault GL and Taylor W, 1982. J. Phys. C. 15: 1753.
        doi:10.1088/0022-3719/15/8/021 http://dx.doi.org/10.1088/0022-3719/15/8/021
11. Berko TI, Dovhyi YaO, Kityk IV, Burak YaV, Djahla VI and Moroz IE, 1993. Ukr. Fiz. Zhurn. 38: 39.
12. Nakamoto K, 1991. Infrared spectra and Raman spectra of inorganic and coordination compounds. Mir. Moscow.
13. Morozov VP, Dergachov MP and Lasunin MV, 2003. Zhurn. Strukturn. Khimiyi 44: 1052.
14. Radaev SF, Muradyan LA, Malachova LF, Burak YaV and Simonov VI, 1989. Kristallogr. 34: 1400.
15. Korshunov AV and Sechkarev AV, 1978. In ‘Modern problems of Raman light spectroscopy’. Nauka, Moscow.
16. Kosevitsh AM, 1981. Physical mechanics of real crystals. Naukova dumka, Kiev.

(c) Ukrainian Journal of Physical Optics